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Concurrent magnetic and structural reconstructions at the interface of (111)-oriented L a0.7 S r0.3Mn O3/LaFe O3

Sammendrag

We observe an induced switchable magnetic moment of
1.6
±
0.40
μ
B
/
Fe
for the nominally antiferromagnetic
LaFe
O
3
extending two to four interface layers into the non–charge transfer system
L
a
0.7
S
r
0.3
Mn
O
3
/
LaFe
O
3
/
SrTi
O
3
(
111
)
. Simultaneously a mismatch of oxygen octahedra rotations at the interface implies an atomic reconstruction of reduced symmetry at the interface, reaching two to five layers into
LaFe
O
3
. Density functional theory of a structure with atomic reconstruction and different correlation strength shows a ferrimagnetic state with a net Fe moment at the interface. Together these results suggest that engineered oxygen octahedra rotations, affecting the local symmetry, affect electron correlations and can be used to promote magnetic properties.

Kategori

Vitenskapelig artikkel

Oppdragsgiver

  • Sigma2 / NN9301K
  • Research Council of Norway (RCN) / 231290

Språk

Engelsk

Forfatter(e)

  • Ingrid Hallsteinsen
  • Magnus Moreau
  • A Grutter
  • Martin Nord
  • Per Erik Vullum
  • DA Gilbert
  • Torstein Bolstad
  • Jostein Grepstad
  • Randi Holmestad
  • Sverre Magnus Selbach
  • AT N'Diaye
  • BJ Kirby
  • E Arenholz
  • Per Thomas Martin Tybell

Institusjon(er)

  • Norges teknisk-naturvitenskapelige universitet
  • Lawrence Berkeley National Laboratory
  • USA
  • SINTEF Industri / Materialer og nanoteknologi

År

2016

Publisert i

Physical Review B. Condensed Matter and Materials Physics

ISSN

1098-0121

Årgang

94

Hefte nr.

20

Side(r)

201115-1 - 201115-6

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